July 16, 2015

New family of chemical structures can effectively remove CO2 from gas mixtures



(July 16, 2015)  A newly discovered family of chemical structures, published in Nature, could increase the value of biogas and natural gas that contains carbon dioxide. The new chemical structures, known as zeolites, have been created by an international team of researchers including Professor Xiaodong Zou and co-workers from the Department of Materials and Environmental Chemistry at Stockholm University.

The zeolites — crystalline aluminosilicates with frameworks that contain windows and cavities the size of small molecules — can separate out carbon dioxide more effectively from fuel gases than those previously known.

Existing zeolites have widespread use in industrial processes that involve gas separation and catalytic conversion, for example to remove nitrogen and carbon dioxide from compressed air to generate oxygen in hospitals and airplanes. There is an ongoing search for new zeolites to add to those known, to augment the small number of different types used commercially.

Highly complex zeolites with attractive properties as adsorbents

However, although many millions of novel structures are both hypothetically possible and energetically feasible, not enough is known about their formation mechanism to prepare them on demand. Rather, new materials are discovered via exploratory synthesis as microcrystalline powders and their structures solved by time-consuming, non-routine approaches.

In the new research published in Nature, research groups from Korea, Sweden and the United Kingdom, have combined structure solution and prediction with targeted synthesis to prepare a family of novel, highly complex zeolites, which have attractive properties as adsorbents.


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