February 1, 2016

Perovskite-nanotubes take light sensitivity to new heights



 Illustration of the perovskite-enhanced photodetector. © E.Horvath (EPFL)

 (February 1, 2016)  EPFL scientists build the most sensitive carbon nanotube-based photodetector to date. The material is sensitized with CN3NH3PbI3 perovskite nanowires, which propel its responsivity by almost seven orders of magnitude.

Semiconducting carbon nanotubes are often used in photovoltaic and optoelectronic devices. But light detection with pristine carbon-nanotube field-effect phototransistors so far is limited in the range of 10% quantum efficiency. The responsivity of the best carbon nanotube devices is around 0.1 A/W. Publishing in Nanoscale, EPFL scientists have now fabricated a carbon-nanotube photodetector with responsivity as high as 7.7×105 A/W.

The lab of László Forró, led by postdocs Bálint Náfrádi and Endre Horváth, at EPFL built the device and overlaid it with perovskite (CN3NH3PbI3) nanowires to sensitize its light-detection capacity. The unprecedented high performance is a result of the two materials working together: the perovskite nanowires can convert incoming light into free charge-carriers with high efficiency, while the carbon nanotube transfers the electrons to the detection circuit.


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